As you know the amount of overlap you have will pretty much dictate how the engine sounds and idles. So it sounds like a tight LSA is the way to go in your case.
There's no doubt a 104 LSA along with low 260's duration would really give you that 60's race car sound.
It does make the engine a little hard to tune for the street and it will of course be harder on gas, but I'm sure it'll make great power.
I've noticed that a lot of the Engine Masters engines use tight LSA's with good results and David Vizard often points out that most builders tend to use LSA's that are too wide for maximum performance.
104 is really tight though. I think it'll work well and sound radical but I'm not sure I'd go much past 256 int. 262 ext. on a 104 LSA. but that's just an opinion based on no real experience with that much duration on a tight LSA. (be sure to check your piston to valve clearance)
I did help a guy I know spec out a 230/236, 106 LSA for a 476 ci. stroker and he loved it.
He wanted a bit of a lopey idle and good midrange but didn't want to rev the engine much past 5,200 rpm.
Joe Sherman used a 265/270 on a 108 LSA for the 437 ci. stroked 348 in this article. It peaked at 6,900 rpm.
http://www.hotrod.com/how-to/engine/hrdp-0911-chevy-w-series-engine-build/
I bought that engine from Joe and I can assure you that it idled like a race engine.
It had 51.5 degrees of overlap. If you went with 256/263 on a 104 LSA you'd have the exact same amount of overlap. I would expect it idle much the same but the horsepower would of course peak at a lower rpm, like maybe 6,300 or 6,400? and maybe shift at about 6,500 or 6,600?
Oddly enough, when I put together the new engine I'm running in the 55 Chevy, I went in the opposite direction. I wanted a smoother idle and didn't need any midrange because of the 6,000 rpm torque converter, so I went with a 112 LSA cam. (263/274 @ .050)
That's "only" 44.5 degrees of overlap so it idles pretty smooth by race car standards.
You might be the first one on the site to use a 104 LSA if you go that way.
I'm thinking it might be just the thing for what you're aiming for. I'm pretty sure it'll work as long as you don't get carried away with the duration.